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Optical properties of the langasite family crystals: La3Ga5SiO14, La3Ga5.5Ta0.5O14, Ca3TaGa3Si2O14
Russian version
DOI: 10.61011/EOS.2023.05.56511.67-22
Zabelina E.V. 1, Kozlova N.S. 1, Buzanov O.A. 2
1National University of Science and Technology MISiS, Moscow, Russia
2FOMOS-Materials, Moscow, Russia
Email: zabelina.ev@misis.ru, kozlova_nina@mail.ru, buzanov@newpiezo.com
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Optical properties of lanthanum-gallium silicate (La3Ga5SiO14), lanthanum-gallium tantalate (La3Ga5.5Ta0.5O14), calcium-tantalum-gallium silicate (Ca3TaGa3Si2O14) crystals in the near ultraviolet (UV) and visible wavelength ranges (200-800 nm) have been studied. For the first time the angles of deviation of the moments of the dipole transition spectral dependences theta(λ) were used to characterize the absorption processes in these crystals. These dependences make it possible to reveal absorption bands that are weakly noticeable on the transmission coefficients spectral dependences, and to estimate the degree of deviation of the dispersion dependence theta(λ) from the value theta=45o corresponding to an ideal ordered crystal. Analysis of theta(λ) dependencies showed that in the studied wavelength range, the lowest deviation from theta=45o is observed in Ca3TaGa3Si2O14, and the highest in La3Ga5SiO14. The coefficients of the specific rotation angle of the polarization plane rho were obtained by the spectrophotometric interference method in polarized light. The measured values are best approximated by the Vyshin equation. For the first time, dependences of the modified Drude formula 1/rho=f(λ2 were calculated for these crystals. These dependences should be linear in case of an ideal crystal. The largest deviation from the linear dependence is observed for La3Ga5SiO14 crystals, and the lowest for Ca3TaGa3Si2O14. The discrete values of the refractive coefficients No and Ne were measured by the prism method. La3Ga5.5Ta0.5O14 crystals have the highest refractive coefficients, Ca3TaGa3Si2O14 crystals have the lowest. The obtained values are approximated by the Sellmeier equation. Keywords: lanthanum-gallium silicate, lanthanum-gallium tantalate, calcium-tantalum-gallium silicate, refractive index, transmission coefficients spectral dependences, polarization plane specific rotation, dipole moment of transition. DOI: 10.61011/EOS.2023.05.56511.67-22
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