Optics and Spectroscopy
To authors
YAl3(BO3)4:Cr crystals for luminescent cryothermometry
Molchanova A. D.
1, Diab M.1,2, Boldyrev K.N.1, Popova M.N.
1
1Institute of Spectroscopy, Russian Academy of Sciences, Troitsk, Moscow, Russia
2Moscow Institute of Physics and Technology (National Research University), Dolgoprudny, Moscow Region, Russia
2Moscow Institute of Physics and Technology (National Research University), Dolgoprudny, Moscow Region, Russia
Email: nastyamolchanova@list.ru, popova@isan.troitsk.ru
The luminescence spectra of the YAl3(BO3)4:Cr3+ crystal have been registered in the spectral range of 2E->4A2 electronic transitions in Cr3+ ions (14550-14700 cm-1) with high spectral resolution at temperatures 4-300 K. The temperature dependences of the ratios of the integral intensities of lines R2 and R1, as well as N' and N (presumably the lines of the 2E->4A2 transitions of the Cr3+ center in a position distorted due to the vicinity of a some defect), correspond well to the Boltzmann distribution. On the measurement of these ratios, a ratiometric thermometer with a maximum absolute sensitivity at temperatures 40.3 and 21.6 K, respectively, and a relative sensitivity of up to 12% K-1 can be realized. Measuring the width of the most intense spectral component - line R1 - can be a way to capture temperature in the range of 100 K and above. Keywords: luminescent cryothermometry, YAl3(BO3)4:Cr3+ crystal, high-resolution Fourier-transform spectroscopy.
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