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VUV-luminescence and excitation spectra of the heavy trivalent rare earth ions in fluoride matrices

Kirm M.^1,2, Makhov V.N.³, True M.¹, Vielhauer S.¹, Zimmerer G.¹

¹Institut fur Experimentalphysik der Universitat Hamburg, Hamburg, Germany
²Institute of Physics, University of Tartu, Tartu, Estonia

³P.N. Lebedev Physical Institute, Russian Academy of Sciences, Moscow, Russia

Email: georg.zimmerer@desy.de

Выставление онлайн: 20 июля 2005 г.

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VUV 4fⁿ->4f^n-15d transitions of Gd³⁺, Er³⁺, Tm³⁺, and Lu³⁺ in fluoride matrices have been analysed with high-resolution luminescence and excitation spectroscopy. In trifluorides, strong electron-phonon coupling has been found. In the other matrices, the luminescence spectra clearly yield zero-phonon lines and phonon replica, indicating intermediate coupling. The energies of the zero-phonon lines observed are compared with theoretical predictions. Near the threshold of f-> d excitations, some of the excitation spectra yield sharp structures which cannot be explained with phonon replica but will be discussed in terms of the energy levels of the 4f^n-15d configuration. The work was supported by the Minister of Science and Technology of Germany under contracts 05 KS1GUD/1 and 03N8019D. Support by the Graduiertenkolleg Felder und lokalisierte Atome-Atome und lokalisierte Felder of the Deutsche Forschungsgemeinschaft (GRK 403) is gratefully acknowledged.

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