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Phase transitions in hydrofullerene C₆₀H₃₆ studied by luminescence and Raman spectroscopy at pressure up to 12 GPa

Meletov K.P.^1,2, Assimopoulos S.¹, Kourouklis G.A.¹, Bashkin I.O.²

¹Physics Division, School of Technology, Aristotle University of Thessaloniki, GR-540 06 Thessaloniki, Greece
²Institute of Solid State Physics, Russian Academy of Sciences, Chernogolovka, Russia

Institute of Solid State Physics, Russian Academy of Sciences, Chernogolovka, Russia

Email: mele@issp.ac.ru

Выставление онлайн: 17 февраля 2002 г.

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The effect of hydrostatic pressure on the photoluminescence and Raman spectra of hydrofullerene C₆₀H₃₆ has been investigated for pressure up to 12 GPa at room temperature. The samples were synthesized by means of high-pressure hydrogenation. The pressure coefficients of the phonon modes are positive and demonstrate singularities at ~ 0.7 and ~ 6 GPa. The pressure shift of the luminescence spectrum is unusually small and increases somehow at P>=q 6 GPa. All observed features are reversible with pressure and C₆₀H₃₆ is stable in the pressure region investigated. This work was supported, in part, by the Russian Foundation for Fundamental Research (grants N 99-02-17555 and 99-02-17299), and the Russian Research and Development Program "Fullerenes and Atomic Clusters" (grant N 98079). The support by the General Secretariat for Research and Technology, Greece (grant N ПENEDelta 99, 99EDelta/62) is acknowledged.

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