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Spectroscopic parameters of LVM absorption bands of carbon and oxygen impurities in isotopic enriched silicon ²⁸Si, ²⁹Si and ³⁰Si

Sennikov P.G.¹, Kotereva T.V.¹, Kurganov A.G.¹, Andreev B.A.¹, Niemann H.¹, Schiel D.¹, Emtsev V.V.¹, Pohl H.-J.¹

¹Institute of Chemistry of High-Purity Substances, Russian Academy of Sciences, Nizhny Novgorod, Russia

Поступила в редакцию: 4 августа 2004 г.

Выставление онлайн: 17 февраля 2005 г.

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The IR spectra of all three Si isotopes in the form of bulk single crystals (²⁸Si with enrichment more as 99.9%, ²⁹Si and ³⁰Si with enrichment more than 90%) has been studied at T=300, 17 and 5 K in spectral range 550-1200 cm^-1. IR active local vibrational modes (LVM) of the Si-¹²C centered at 605 cm^-1 and of Si-¹⁶O-Si quasi-molecules in region of 1136 cm^-1 for all Si isotopes in comparison with Si of natural isotopic composition as well as its isotopic shift at 300 and 17 K have been determined. The dependence of shape of antisymmetric stretching vibration band of ²⁸Si-¹⁶O-²⁸Si in spectrum of ²⁸Si on spectral resolution has been studied. The perspectives of generalization of IR spectroscopy method for determination of carbon and oxygen impurities in Si of natural isotopic composition to mono-isotopic Si have been discussed.

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